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Found 10489 publications. Showing page 364 of 420:

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Mobile monitoring of urban ultrafine particles in Novi Sad, Serbia

Davidović, Miloš D.; Kleut, Duška N.; Vito, Saverio De; Bartonova, Alena; Jovasevic-Stojanovic, Milena

2023

A high-resolution dynamic probabilistic material flow analysis of seven plastic polymers; A case study of Norway

Abbasi, Golnoush; Hauser, Marina Jennifer; Baldé, Cornelis Peter; Bouman, Evert Alwin

Plastic pollution has long been identified as one of the biggest challenges of the 21st century. To tackle this problem, governments are setting stringent recycling targets to keep plastics in a closed loop. Yet, knowledge of the stocks and flows of plastic has not been well integrated into policies. This study presents a dynamic probabilistic economy-wide material flow analysis (MFA) of seven plastic polymers (HDPE, LDPE, PP, PS, PVC, EPS, and PET) in Norway from 2000 to 2050. A total of 40 individual product categories aggregated into nine industrial sectors were examined. An estimated 620 ± 23 kt or 114 kg/capita of these seven plastic polymers was put on the Norwegian market in 2020. Packaging products contributed to the largest share of plastic put on the market (∼40%). The accumulated in-use stock in 2020 was about 3400 ± 56 kt with ∼60% remaining in buildings and construction sector. In 2020, about 460 ± 22 kt of plastic waste was generated in Norway, with half originating from packaging. Although ∼50% of all plastic waste is collected separately from the waste stream, only around 25% is sorted for recycling. Overall, ∼50% of plastic waste is incinerated, ∼15% exported, and ∼10% landfilled. Under a business-as-usual scenario, the plastic put on the market, in-use stock, and waste generation will increase by 65%, 140%, and 90%, respectively by 2050. The outcomes of this work can be used as a guideline for other countries to establish the stocks and flows of plastic polymers from various industrial sectors which is needed for the implementation of necessary regulatory actions and circular strategies. The systematic classification of products suitable for recycling or be made of recyclate will facilitate the safe and sustainable recycling of plastic waste into new products, cap production, lower consumption, and prevent waste generation.

2023

The influence of vegetation drought stress on formaldehyde and ozone distributions over a central European city

Trimmel, Heidelinde; Hamer, Paul David; Mayer, Monika; Schreier, Stefan F.; Weihs, Philipp; Eitzinger, Josef; Sandén, Hans; Fitzky, Anne Charlott; Richter, Andreas; Calvet, Jean-Christophe; Bonan, Bertrand; Meurey, Catherine; Vallejo, Islen; Eckhardt, Sabine; Santos, Gabriela Sousa; Oumami, Safae; Arteta, Joaquim; Marécal, Virginie; Tarrasón, Leonor; Karl, Thomas; Rieder, Harald E.

To estimate the effect of vegetation stress and changes in biogenic volatile organic compound (BVOC) emissions on urban ozone (O3) levels we perform a systematic, observation-based analysis of the relationship between formaldehyde (HCHO) mixing ratios, meteorological parameters, measurement-based drought indicators and O3 over the central European city of Vienna, Austria. In addition, numerical models SURface EXternalisée (SURFEX), Model of Emissions of Gases and Aerosols from Nature (MEGAN) Vers.2.1 and 3 and MOdèle de Chimie A Grande Echelle (MOCAGE) are combined to estimate the soil moisture, the spatial distribution and drought response of isoprene emissions, and the resulting distribution of HCHO in the atmosphere. To analyse the effect of drought during spring and summer we contrast observations during dry and reference years. Our results show that the observed HCHO can be explained using the simulated isoprene emissions as well as observed and simulated vegetation drought responses. HCHO mixing ratios differ strongly between dry and reference seasons. Spring-time precipitation deficits facilitate reduced HCHO mixing ratios due to delayed and weakened plant growth. In consequence also O3 burdens are lowered due to reduced BVOC precursor emissions. These reductions occur despite radiation levels being higher than during the reference year, illustrating the strong potential of spring-time BVOC emissions to modulate urban O3 burdens. Conversely, during summer elevated O3 levels occur during local drought conditions. These are driven by advected isoprene originating from nearby forest areas, which are not affected by drought. Our results regarding elevated summer-time O3 burdens under vegetation heat and drought stress are in good agreement with previous work.

2023

Chlorinated paraffins in urban air in Nordic countries

Bohlin-Nizzetto, Pernilla; Borgen, Anders; Nipen, Maja

In 2022, the Joint Nordic screening group decided to perform a Nordic study on short-, medium- and long-chain chlorinated paraffins (SCCPs, MCCPs, LCCPs) in urban air. A previous study performed on behalf of screening group in 2019 observed higher concentrations of chlorinated paraffins (CPs) in air samples from an urban site than from remote sites (Schlabach et al. 2022). It was then suggested that tire wear particles could be the source for the elevated urban concentrations.

The focus of the study in 2022 was to collect data to improve the understanding of sources for CPs in air by: (1) comparing concentrations measured in wintertime when studded tires are used and in summertime when normal tires are used, (2) comparing data from three capitals in the Nordic countries, and (3) compare urban air concentrations to air concentrations in a car tire testing facility. All the member countries were invited to participate but based on the possibilities to collect active air samples in urban locations, it was decided to collect air samples from Helsinki (Finland), Reykjavik and Reykjanesbær (Iceland) and Oslo (Norway). Samples were collected in February–March 2022 and May–August 2022. The sampling time for each sample was 48 hrs and 3–6 samples were collected per site and season.

Nordic Council of Ministers

2023

Status report of air quality in Europe for year 2021, using validated data

Targa, Jaume; Ripoll, Anna; Banyuls, Lorena; Ortiz, Alberto González; Soares, Joana

ETC/HE

2023

Per- and polyfluoroalkyl substances (PFASs) – An underestimated environmental and analytical challenge

Kallenborn, Roland; Hartz, William Frederik; Björnsdotter, Maria; Ali, Aasim Musa Mohamed; Yeung, Leo WY.

2023

Low-Processing Data Enrichment and Calibration for PM2.5 Low-Cost Sensors

Stojanović, Danka B.; Kleut, Duška N.; Davidović, Miloš D.; Vito, Saverio De; Jovasević-Stojanović, Milena V.; Bartonova, Alena; Lepioufle, Jean-Marie

Particulate matter (PM) in air has been proven to be hazardous to human health. Here we focused on analysis of PM data we obtained from the same campaign which was presented in our previous study. Multivariate linear and random forest models were used for the calibration and analysis. In our linear regression model the inputs were PM, temperature and humidity measured with low-cost sensors, and the target was the reference PM measurements obtained from SEPA in the same timeframe.

2023

Monitoring of environmental contaminants in air and precipitation. Annual report 2022.

Halvorsen, Helene Lunder; Pfaffhuber, Katrine Aspmo; Nipen, Maja; Bohlin-Nizzetto, Pernilla; Berglen, Tore Flatlandsmo; Nikiforov, Vladimir; Hartz, William Frederik

This report presents air monitoring data from 2022 for the Norwegian monitoring programme "Atmospheric contaminants". The results cover 260 organic compounds (regulated and non-regulated) and 16 compound groups, 14 heavy metals, and a selection of organic chemicals of concern.

NILU

2023

Energetic Particle Precipitation reflected in the Global Secondary Ozone Distribution

Jia, Jia; Murberg, Lise Eder; Løvset, Tiril; Orsolini, Yvan Joseph Georges Emile G.; Espy, Patrick Joseph; Salinas, Jude; Lee, Jae N.; Wu, Dong; Zhang, Jiarong

2023

The role of SVOCs in the initial film formation and soiling of unvarnished paintings

Grøntoft, Terje; Cutajar, Jan Dariusz

In recent years increased research efforts and environmental improvements have been directed towards the preventive conservation of the monumental, unvarnished oil paintings on canvas (1909–1916) by Edvard Munch (1863–1944) housed in the University of Oslo Aula. Surface soiling of the paintings has been a documented issue since their display, and the modern-day effect of air-borne particulates and gases on the painting surfaces remains hitherto undocumented. For the first time in the Aula, this study has measured the in-situ time-dependent mass deposit of air pollution onto vertical surfaces over the period of one year (2021–2022). Concomitant measurements of the concentrations of ozone (O3) and nitrogen dioxide (NO2) were also taken, to complement periodic data from 2020. The mass deposit was measured through incremental weight changes of Teflon membrane filters, and quartz filters for analysis of elemental/organic carbon (EC/OC), whilst the gaseous pollutants were measured using passive gas samplers. Indoor-to-outdoor ratios (I/O) for O3 were noted to be higher than those suggested by earlier data, whereas NO2 I/O ratios were found to be lower, indicating a stronger oxidising atmosphere in the Aula. Just over half of the deposited mass on the quartz filters was found to be OC, with no EC detected. Surprisingly, an overall decrease in the mass deposit from three to twelve months was measured on the Teflon membrane filters. It was hypothesised, based on models reported in the literature, that the source of the OC on the filters was mainly gaseous, semi-volatile organic compounds (SVOCs), which were present in an adsorption/desorption equilibrium that was dependent on possible SVOC emission episodes, relative humidity levels, gaseous oxidative reactions and the particulate matter deposit. A simple mathematical model is proposed to rationalise the observed mass deposits on the filters, together with a discussion of uncertainties affecting the measurements. The hypothesis preliminarily indicates the possible and previously unconsidered role of SVOCs on the initial film formation of soiling layers on the Aula paintings, and could bear implications for their monitoring in the preventive care of unvarnished oil paintings on canvas.

2023

Chemical analysis of POPs and heavy metals in precipitation at NILU

Uggerud, Hilde Thelle; Halvorsen, Helene Lunder

2023

Interim air quality maps of EEA member and cooperating countries for 2022. PM10, O3, and NO2 spatial estimates and evaluation of PM2.5 interim mapping.

Horálek, Jan; Vlasakova, Leona; Schreiberova, Marketa; Schneider, Philipp; Benesova, Nina

This report presents European interim air quality maps for 2022, which are based on the non-validated up-to-date (UTD) measurement data and the CAMS Ensemble Forecast modelling results, together with other supplementary data. It contains maps of PM10 annual average, ozone indicator SOMO35 and NO2 annual average. Next to this, the report evaluates the PM2.5 annual mean interim mapping.

ETC/HE

2023

Changes in the atmospheric chemical composition and impacts on climate, health, and ecosystems

Aas, Wenche; Bohlin-Nizzetto, Pernilla; Eckhardt, Sabine; Myhre, Cathrine Lund; Platt, Stephen Matthew; Solberg, Sverre; Svendby, Tove Marit; Tørseth, Kjetil; Yttri, Karl Espen

2023

Global agricultural ammonia emissions simulated with the ORCHIDEE land surface mode

Beaudor, Maureen; Vuichard, Nicolas; Lathière, Juliette; Evangeliou, Nikolaos; Damme, Martin Van; Clarisse, Lieven; Hauglustaine, Didier

Ammonia (NH3) is an important atmospheric constituent. It plays a role in air quality and climate through the formation of ammonium sulfate and ammonium nitrate particles. It has also an impact on ecosystems through deposition processes. About 85 % of NH3 global anthropogenic emissions are related to food and feed production and, in particular, to the use of mineral fertilizers and manure management. Most global chemistry transport models (CTMs) rely on bottom-up emission inventories, which are subject to significant uncertainties. In this study, we estimate emissions from livestock by developing a new module to calculate ammonia emissions from the whole agricultural sector (from housing and storage to grazing and fertilizer application) within the ORCHIDEE (Organising Carbon and Hydrology In Dynamic Ecosystems) global land surface model. We detail the approach used for quantifying livestock feed management, manure application, and indoor and soil emissions and subsequently evaluate the model performance. Our results reflect China, India, Africa, Latin America, the USA, and Europe as the main contributors to global NH3 emissions, accounting for 80 % of the total budget. The global calculated emissions reach 44 Tg N yr−1 over the 2005–2015 period, which is within the range estimated by previous work. Key parameters (e.g., the pH of the manure, timing of N application, and atmospheric NH3 surface concentration) that drive the soil emissions have also been tested in order to assess the sensitivity of our model. Manure pH is the parameter to which modeled emissions are the most sensitive, with a 10 % change in emissions per percent change in pH. Even though we found an underestimation in our emissions over Europe (−26 %) and an overestimation in the USA (+56 %) compared with previous work, other hot spot regions are consistent. The calculated emission seasonality is in very good agreement with satellite-based emissions. These encouraging results prove the potential of coupling ORCHIDEE land-based emissions to CTMs, which are currently forced by bottom-up anthropogenic-centered inventories such as the CEDS (Community Emissions Data System).

2023

Migration analysis of chemical additives from indoor consumer plastic products

Bohlin-Nizzetto, Pernilla

NILU has, on behalf of the Norwegian Environment Agency, performed chemical analyses of a selection of chemical additives in indoor consumer plastic products. The goal was to identify content and migration of the chemical additives in and from the products to particles and surfaces of the products at room temperature. The plastic products included; furniture wrap, wall papers, table cloths, shower curtains, floor tiles, mattresses, pillows, carpet underlays and a bathtub mat. Targeted chemicals were organophosphorous flame retardants (OPFRs), brominated flame retardants (BFRs) including tetrabromobisphenol A (TBBPA), chlorinated paraffins (CPs) and dechloranes. MCCPs and SCCPs were found in ‰ to % levels in PVC containing products. Four of the OPFRs were found in up to ‰ levels in adhesive foils to be put on furniture or floor/walls and mattresses. None of the targeted brominated compounds nor melamine were detected in the product samples.

NILU

2023

Revidert tiltaksutredning for lokal luftkvalitet i Drammen

Weydahl, Torleif; Markelj, Miha; Høyem, Harald

NILU – Norsk institutt for luftforskning har, i samarbeid med Asplan Viak AS, utarbeidet en tiltaksutredning for lokal luftkvalitet i Drammen kommune. Tiltaksutredningen omfatter en kartlegging av luftkvaliteten i Drammen ved trafikkberegninger og utslipps- og spredningsberegninger for svevestøv (PM10 og PM2,5) for Dagens situasjon 2021 og Referansesituasjonen 2030 og for 2030 med tiltak rettet mot svevestøv. Basert på resultatene fra beregningene og i samarbeid med oppdragsgiver, styringsgruppe og referansegruppe, er det foreslått en revidert handlingsplan som skal behandles politisk.

NILU

2023

Kan vi leve uten plast?

Hanssen, Linda (interview subject); Jemterud, Torkild (journalist)

2023

Determination of PFC with Canister Sampling and Medusa GC–MS Analysis in Comparison to General IPCC Estimation Methods

Åsheim, Henrik; Isaksen, Morten; Hermansen, Ove; Schmidbauer, Norbert; Lunder, Chris Rene

2023

Long-term Comparison of NOAA and AGAGE Non-CO2 Trace Gas Observations at Common Sites

Hall, Brad D.; Krummel, Paul B.; Muhle, Jens; Weiss, Ray F.; Montzka, Stephen A.; Vimont, Isaac J.; Dutton, Geoffrey S.; Harth, Christina M.; O'Doherty, Simon; Young, Dickon; nance, Jon David; Loh, Zoe M; Lan, Xin; Langenfelds, Ray; Salameh, Peter K.; Prinn, Ronald G.; Mitrevski, Blagoj; Lunder, Chris Rene

2023

Aerosol and dynamical contributions to cloud droplet formation in Arctic low-level clouds

Motos, Ghislain; Freitas, Gabriel; Georgakaki, Paraskevi; Wieder, Jörg; Li, Guangyu; Aas, Wenche; Lunder, Chris Rene; Krejci, Radovan; Pasquier, Julie Thérèse; Henneberger, Jan; David, Robert Oscar; Ritter, Christoph; Mohr, Claudia; Zieger, Paul; Nenes, Athanasios

The Arctic is one of the most rapidly warming regions of the globe. Low-level clouds and fog modify the energy transfer from and to space and play a key role in the observed strong Arctic surface warming, a phenomenon commonly termed “Arctic amplification”. The response of low-level clouds to changing aerosol characteristics throughout the year is therefore an important driver of Arctic change that currently lacks sufficient constraints. As such, during the NASCENT campaign (Ny-Ålesund AeroSol Cloud ExperimeNT) extending over a full year from October 2019 to October 2020, microphysical properties of aerosols and clouds were studied at the Zeppelin station (475 m a.s.l.), Ny-Ålesund, Svalbard, Norway. Particle number size distributions obtained from differential mobility particle sizers as well as chemical composition derived from filter samples and an aerosol chemical speciation monitor were analyzed together with meteorological data, in particular vertical wind velocity. The results were used as input to a state-of-the-art cloud droplet formation parameterization to investigate the particle sizes that can activate to cloud droplets, the levels of supersaturation that can develop, the droplet susceptibility to aerosol and the role of vertical velocity. We evaluate the parameterization and the droplet numbers calculated through a droplet closure with in-cloud in situ measurements taken during nine flights over 4 d. A remarkable finding is that, for the clouds sampled in situ, closure is successful in mixed-phase cloud conditions regardless of the cloud glaciation fraction. This suggests that ice production through ice–ice collisions or droplet shattering may have explained the high ice fraction, as opposed to rime splintering that would have significantly reduced the cloud droplet number below levels predicted by warm-cloud activation theory. We also show that pristine-like conditions during fall led to clouds that formed over an aerosol-limited regime, with high levels of supersaturation (generally around 1 %, although highly variable) that activate particles smaller than 20 nm in diameter. Clouds formed in the same regime in late spring and summer, but aerosol activation diameters were much larger due to lower cloud supersaturations (ca. 0.5 %) that develop because of higher aerosol concentrations and lower vertical velocities. The contribution of new particle formation to cloud formation was therefore strongly limited, at least until these newly formed particles started growing. However, clouds forming during the Arctic haze period (winter and early spring) can be limited by updraft velocity, although rarely, with supersaturation levels dropping below 0.1 % and generally activating larger particles (20 to 200 nm), including pollution transported over a long range. The relationship between updraft velocity and the limiting cloud droplet number agrees with previous observations of various types of clouds worldwide, which supports the universality of this relationship.

2023

Atmospheric Microplastic in the Arctic and the Norwegian mainland

Gossmann, Isabel; Herzke, Dorte; Nikiforov, Vladimir; Held, Andreas; Schulz, Janina; Georgi, Christoph; Evangeliou, Nikolaos; Eckhardt, Sabine; Gerdts, Gunnar; Wurl, Oliver; Scholz-Böttcher, Barbara

2023

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