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Found 9895 publications. Showing page 379 of 396:

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Unchanged PM2.5 levels over Europe during COVID-19 were buffered by ammonia

Evangeliou, Nikolaos; Tichý, Ondřej; Otervik, Marit Svendby; Eckhardt, Sabine; Balkanski, Yves; Hauglustaine, Didier A.

The coronavirus outbreak in 2020 had a devastating impact on human life, albeit a positive effect on the environment, reducing emissions of primary aerosols and trace gases and improving air quality. In this paper, we present inverse modelling estimates of ammonia emissions during the European lockdowns of 2020 based on satellite observations. Ammonia has a strong seasonal cycle and mainly originates from agriculture. We further show how changes in ammonia levels over Europe, in conjunction with decreases in traffic-related atmospheric constituents, modulated PM2.5. The key result of this study is a −9.8 % decrease in ammonia emissions in the period of 15 March–30 April 2020 (lockdown period) compared to the same period in 2016–2019, attributed to restrictions related to the global pandemic. We further calculate the delay in the evolution of the ammonia emissions in 2020 before, during, and after lockdowns, using a sophisticated comparison of the evolution of ammonia emissions during the same time periods for the reference years (2016–2019). Our analysis demonstrates a clear delay in the evolution of ammonia emissions of −77 kt, which was mainly observed in the countries that imposed the strictest travel, social, and working measures. Despite the general drop in emissions during the first half of 2020 and the delay in the evolution of the emissions during the lockdown period, satellite and ground-based observations showed that the European levels of ammonia increased. On one hand, this was due to the reductions in SO2 and NOx (precursors of the atmospheric acids with which ammonia reacts) that caused less binding and thus less chemical removal of ammonia (smaller loss – higher lifetime). On the other hand, the majority of the emissions persisted because ammonia mainly originates from agriculture, a primary production sector that was influenced very little by the lockdown restrictions. Despite the projected drop in various atmospheric aerosols and trace gases, PM2.5 levels stayed unchanged or even increased in Europe due to a number of reasons that were attributed to the complicated system. Higher water vapour during the European lockdowns favoured more sulfate production from SO2 and OH (gas phase) or O3 (aqueous phase). Ammonia first reacted with sulfuric acid, also producing sulfate. Then, the continuously accumulating free ammonia reacted with nitric acid, shifting the equilibrium reaction towards particulate nitrate. In high-free-ammonia atmospheric conditions such as those in Europe during the 2020 lockdowns, a small reduction in NOx levels drives faster oxidation toward nitrate and slower deposition of total inorganic nitrate, causing high secondary PM2.5 levels.

2025

Uncovering transport, deposition and impact of radionuclides released after the early spring 2020 wildfires in the Chernobyl Exclusion Zone

Evangeliou, Nikolaos; Eckhardt, Sabine

In the beginning of April 2020, large fires that started in the Chernobyl Exclusion Zone (CEZ) established after the Chernobyl accident in 1986 caused media and public concerns about the health impact from the resuspended radioactivity. In this paper, the emissions of previously deposited radionuclides from these fires are assessed and their dispersion and impact on the population is examined relying on the most recent data on radioactive contamination and emission factors combined with satellite observations. About 341 GBq of 137Cs, 51 GBq of 90Sr, 2 GBq of 238Pu, 33 MBq of 239Pu, 66 MBq of 240Pu and 504 MBq of 241Am were released in 1st–22nd April 2020 or about 1,000,000,000 times lower than the original accident in 1986 and mostly distributed in Central and East Europe. The large size of biomass burning particles carrying radionuclides prevents long-range transport as confirmed by concentrations reported in Europe. The highest cumulative effective doses (> 15 μSv) were calculated for firefighters and the population living in the CEZ, while doses were much lower in Kiev (2–5 μSv) and negligible in Belarus, Russia and Europe. All doses are radiologically insignificant and no health impact o

Nature Portfolio

2020

Underestimation of Anthropogenic Bromoform Emissions: Implications for Ozone Depletion

Jia, Yue; Davis, Sean M; Tegtmeier, Susann; Quack, Birgit; Pisso, Ignacio; Portmann, Robert W.; Rosenlof, Karen H.

2023

Understand and mitigate impacts of 3D clouds on UV-VIS NO2 trace gas retrievals by AI exploration of synthetic and real data

Kylling, Arve; Emde, Claudia; Yu, Huan; van Roozendael, Michel; Stebel, Kerstin; Mayer, Bernhard

2022

2000

Understanding Air Quality Trends in Europe. Focus on the relative contribution of changes in emission of activity sectors, natural fraction and meteorological variability.

Colette, Augustin; Solberg, Sverre; Aas, Wenche; Walker, Sam-Erik

Emission changes are the main driver of all air pollutant trends. For NO2 and PM10, both the GAM and the CTM results indicate that emission changes contribute to at least 90% of the 2000-2017 trend. For ozone peaks (as 4MDA8), meteorology can be important. The GAM model estimates that it contributes to an increase counteracting mitigation effort up to a magnitude of 20 to 80% (compared to the effect of emission and background changes) in Austria, Belgium, Czech Republic, France, and Italy. Given the good skill of the GAM model to capture meteorological effect, this estimate can be considered quite robust.

The relative contribution of agriculture and industry to the total PM10 mass has been reduced by around 30% for both sectors, but the similarity of evolution is not directly linked to the emission trends in the respective sectors. The relationship between emissions and concentrations is nonlinear and depends on availability of precursor gases to form ammonium sulphate and ammonium nitrate. The relative contribution of traffic sources to PM10 has been reduced with around 20%, while the trend attributed to residential heating is marginal. The heating sector has become a relatively more important contributor to the aerosol pollution and needs more attention. The model also indicates that the natural contributions (such as sea salt and dust) has had little impact on the long-term changes in PM10.

The analysis includes observational data only from stations with data available for at least 14 years in the period 2000-2017. This drastically reduces the number of monitoring sites included in the analysis and the spatial representativity of the assessment, with bias towards countries benefiting from a long-term monitoring network.

Further improvements of models as well as observational basis are needed to reduce the uncertainties. Understanding organic aerosols from the residential heating sector should be a priority.

ETC/ATNI

2021

Understanding individual heat exposure through interdisciplinary research on thermoception

Serrano, Paloma Yáñez; Bieńkowska, Zofia; Boni, Zofia; Chwałczyk, Franciszek; Hassani, Amirhossein

Extreme heat events are more frequent and more intense globally due to climate change. The urban environment is an additional factor enhancing the effects of heat. Adults above 65 years old are especially at risk due to their poorer health, physiology and socio-economic situation. Yet, there is limited knowledge about their experiences of summer heat, their actual heat exposure and how they negotiate their thermal comfort through different adaptation practices. In conventional research on heat exposure and thermal comfort, very little attention is given to individual behaviour and subjective experiences. To understand how older adults feel the heat in the city we study their thermoception, which we conceptualise as an embodied knowledge about bodily sensations, thermal environments and adjustments to heat. This article stems from interdisciplinary research conducted in Warsaw and Madrid in the summers of 2021–2022. We combine and juxtapose data from ethnographic research and from physical measurements of temperature gathered in people’s homes, to show on a microscale how we can study and understand the diversity in individual heat exposure more holistically. We demonstrate that to understand the consequences of heat for vulnerable populations it is crucial to study thermoception, the subjective experiences of heat, in addition to analysing their thermal environments. With the use of a unique methodology, this article shows how similar weather conditions are experienced differently by people from the same cities, depending on the materiality of their dwellings, availability of cooling devices, as well as everyday habits and their individual bodies. We discuss the social, material and temporal adjustments participants made to deal with heat, to showcase their agency in affecting their individual heat exposure. The article emphasises the role of social sciences and qualitative methods in research on individual heat exposure and argues for the co-production of knowledge on the topic.

Palgrave Macmillan

2024

Understanding of European cold extremes, sudden stratospheric warming, and Siberian snow accumulation in the winter of 2017/18

Lü, Zhuozhuo; Li, Fei; Orsolini, Yvan; Gao, Yongqi; He, Shengping

It is unclear whether the Eurasian snow plays a role in the tropospheric driving of sudden stratospheric warming (SSW). The major SSW event of February 2018 is analyzed using reanalysis datasets. Characterized by predominant planetary waves of zonal wave 2, the SSW developed into a vortex split via wave–mean flow interaction. In the following two weeks, the downward migration of zonal-mean zonal wind anomalies was accompanied by a significant transition to the negative phase of the North Atlantic Oscillation, leading to extensive cold extremes across Europe. Here, we demonstrate that anomalous Siberian snow accumulation could have played an important role in the 2018 SSW occurrence. In the 2017/18 winter, snow depths over Siberia were much higher than normal. A lead–lag correlation analysis shows that the positive fluctuating snow depth anomalies, leading to intensified “cold domes” over eastern Siberia (i.e., in a region where the climatological upward planetary waves maximize), precede enhanced wave-2 pulses of meridional heat fluxes (100 hPa) by 7–8 days. The snow–SSW linkage over 2003–19 is further investigated, and some common traits among three split events are found. These include a time lag of about one week between the maximum anomalies of snow depth and wave-2 pulses (100 hPa), high sea level pressure favored by anomalous snowpack, and a ridge anchoring over Siberia as precursor of the splits. The role of tropospheric ridges over Alaska and the Urals in the wave-2 enhancement and the role of Arctic sea ice loss in Siberian snow accumulation are also discussed.

American Meteorological Society (AMS)

2020

Understanding the exposure pathways of per- and polyfluorinated chmicals (PFC) via use of PFC-containing products - risk estimation for man and environment. NILU F

Knepper, T.P.; Frömel, T.; Gremmel, C.; van Driezum, I.; Weil, H.; Vestergren, R.; Cousins, I.T.

2013

Understanding the fate and bioaccumulation of cyclic volatile methyl siloxanes (cVMS) in Arctic lakes.

Krogseth, I.S.; Warner, N.A.; Breivik, K.; Whealan, M.; Evenset, A.; Christensen, G.N.; Wassbotten, I.H.

2014

Understanding the fate and bioaccumulation of cyclic volatile methyl siloxanes (cVMS) in Arctic lakes. NILU PP

Krogseth, I.,Warner, N.A.; Christensen, G.N.; Whelan, M.J.; Breivik, K.; Evenset, A.; Wasbotten, I.H.

2014

Understanding the fate and bioaccumulation of cyclic volatile methyl siloxanes (cVMS) in Arctic lakes. NILU F

Krogseth, I.,Warner, N.A.; Christensen, G.N.; Whelan, M.J.; Breivik, K.; Evenset, A.; Wasbotten, I.H.

2014

Understanding the fate and bioaccumulation of cyclic volatile methyl siloxanes in an Arctic lake.

Krogseth, I.; Warner, N.; Christensen,G.; Whelan, M.; Breivik, K.; Evenset, A.; Wasbotten, I.

2015

Understanding the fate and bioaccumulation of cyclic volatile methyl siloxanes in an Arctic lake.

Krogseth, I.; Warner, N.; Christensen,G.; Whelan, M.; Breivik, K.; Evenset, A.; Wasbotten, I.

2015

Understanding the fate and bioaccumulation of cyclic volatile methyl siloxanes in Arctic lakes.

Krogseth, I.,Warner, N.A.; Christensen, G.N.; Whelan, M.J.; Breivik, K.; Evenset, A.; Wasbotten, I.H.

2014

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