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Found 2670 publications. Showing page 89 of 267:

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Primary aerosol and secondary inorganic aerosol budget over the Mediterranean Basin during 2012 and 2013

Guth, Jonathan; Marécal, Virginie; Josse, Béatrice; Arteta, Joaquim; Hamer, Paul

In the frame of the Chemistry-Aerosol Mediterranean Experiment (ChArMEx), we analyse the budget of primary aerosols and secondary inorganic aerosols over the Mediterranean Basin during the years 2012 and 2013. To do this, we use two year-long numerical simulations with the chemistry-transport model MOCAGE validated against satellite- and ground-based measurements. The budget is presented on an annual and a monthly basis on a domain covering 29 to 47° N latitude and 10° W to 38° E longitude.

The years 2012 and 2013 show similar seasonal variations. The desert dust is the main contributor to the annual aerosol burden in the Mediterranean region with a peak in spring, and sea salt being the second most important contributor. The secondary inorganic aerosols, taken as a whole, contribute a similar level to sea salt. The results show that all of the considered aerosol types, except for sea salt aerosols, experience net export out of our Mediterranean Basin model domain, and thus this area should be considered as a source region for aerosols globally. Our study showed that 11 % of the desert dust, 22.8 to 39.5 % of the carbonaceous aerosols, 35 % of the sulfate and 9 % of the ammonium emitted or produced into the study domain are exported. The main sources of variability for aerosols between 2012 and 2013 are weather-related variations, acting on emissions processes, and the episodic import of aerosols from North American fires.

In order to assess the importance of the anthropogenic emissions of the marine and the coastal areas which are central for the economy of the Mediterranean Basin, we made a sensitivity test simulation. This simulation is similar to the reference simulation but with the removal of the international shipping emissions and the anthropogenic emissions over a 50 km wide band inland along the coast. We showed that around 30 % of the emissions of carbonaceous aerosols and 35 to 60 % of the exported carbonaceous aerosols originates from the marine and coastal areas. The formation of 23, 27 and 27 %, respectively of, ammonium, nitrate and sulfate aerosols is due to the emissions within the marine and coastal area.

2018

Mineral Dust Instantaneous Radiative Forcing in the Arctic

Kylling, Arve; Zwaaftink, Christine Groot; Stohl, Andreas

2018

Comparison of dust-layer heights from active and passive satellite sensors

Kylling, Arve; Vandenbussche, Sophie; Capelle, Virginie; Cuesta, Juan; Klüser, Lars; Lelli, Luca; Popp, Thomas; Stebel, Kerstin; Veefkind, Pepijn

Aerosol-layer height is essential for understanding the impact of aerosols on the climate system. As part of the European Space Agency Aerosol_cci project, aerosol-layer height as derived from passive thermal and solar satellite sensors measurements have been compared with aerosol-layer heights estimated from CALIOP measurements. The Aerosol_cci project targeted dust-type aerosol for this study. This ensures relatively unambiguous aerosol identification by the CALIOP processing chain. Dust-layer height was estimated from thermal IASI measurements using four different algorithms (from BIRA-IASB, DLR, LMD, LISA) and from solar GOME-2 (KNMI) and SCIAMACHY (IUP) measurements. Due to differences in overpass time of the various satellites, a trajectory model was used to move the CALIOP-derived dust heights in space and time to the IASI, GOME-2 and SCIAMACHY dust height pixels. It is not possible to construct a unique dust-layer height from the CALIOP data. Thus two CALIOP-derived layer heights were used: the cumulative extinction height defined as the height where the CALIOP extinction column is half of the total extinction column, and the geometric mean height, which is defined as the geometrical mean of the top and bottom heights of the dust layer. In statistical average over all IASI data there is a general tendency to a positive bias of 0.5–0.8 km against CALIOP extinction-weighted height for three of the four algorithms assessed, while the fourth algorithm has almost no bias. When comparing geometric mean height there is a shift of −0.5 km for all algorithms (getting close to zero for the three algorithms and turning negative for the fourth). The standard deviation of all algorithms is quite similar and ranges between 1.0 and 1.3 km. When looking at different conditions (day, night, land, ocean), there is more detail in variabilities (e.g. all algorithms overestimate more at night than during the day). For the solar sensors it is found that on average SCIAMACHY data are lower by −1.097 km (−0.961 km) compared to the CALIOP geometric mean (cumulative extinction) height, and GOME-2 data are lower by −1.393 km (−0.818 km).

2018

A multi-model comparison of meteorological drivers of surface ozone over Europe

Otero, Noelia; Sillmann, Jana; Mar, Kathleen; Rust, Henning W.; Solberg, Sverre; Andersson, Camilla; Engardt, Magnuz; Bergström, Robert; Bessagnet, Bertrand; Colette, Augustin; Couvidat, Florian; Cuvelier, Cornelius; Tsyro, Svetlana; Fagerli, Hilde; Schaap, Martijn; Manders, Astrid; Mircea, Mihaela; Briganti, Gino; Cappelletti, Andrea; Adani, Mario; D'Isidoro, Massimo; Pay, María Teresa; Theobald, Mark; Vivanco, Marta G.; Wind, Peter; Ojha, Narendra; Raffort, Valentin; Butler, Tim

The implementation of European emission abatement strategies has led to a significant reduction in the emissions of ozone precursors during the last decade. Ground-level ozone is also influenced by meteorological factors such as temperature, which exhibit interannual variability and are expected to change in the future. The impacts of climate change on air quality are usually investigated through air-quality models that simulate interactions between emissions, meteorology and chemistry. Within a multi-model assessment, this study aims to better understand how air-quality models represent the relationship between meteorological variables and surface ozone concentrations over Europe. A multiple linear regression (MLR) approach is applied to observed and modelled time series across 10 European regions in springtime and summertime for the period of 2000–2010 for both models and observations. Overall, the air-quality models are in better agreement with observations in summertime than in springtime and particularly in certain regions, such as France, central Europe or eastern Europe, where local meteorological variables show a strong influence on surface ozone concentrations. Larger discrepancies are found for the southern regions, such as the Balkans, the Iberian Peninsula and the Mediterranean basin, especially in springtime. We show that the air-quality models do not properly reproduce the sensitivity of surface ozone to some of the main meteorological drivers, such as maximum temperature, relative humidity and surface solar radiation. Specifically, all air-quality models show more limitations in capturing the strength of the ozone–relative-humidity relationship detected in the observed time series in most of the regions, for both seasons. Here, we speculate that dry-deposition schemes in the air-quality models might play an essential role in capturing this relationship. We further quantify the relationship between ozone and maximum temperature (mo3 − T, climate penalty) in observations and air-quality models. In summertime, most of the air-quality models are able to reproduce the observed climate penalty reasonably well in certain regions such as France, central Europe and northern Italy. However, larger discrepancies are found in springtime, where air-quality models tend to overestimate the magnitude of the observed climate penalty.

2018

Curating scientific information in knowledge infrastructures

Stocker, Markus; Paasonen, Pauli; Fiebig, Markus; Zaidan, Martha A; Hardisty, Alex

Interpreting observational data is a fundamental task in the sciences, specifically in earth and environmental science where observational data are increasingly acquired, curated, and published systematically by environmental research infrastructures. Typically subject to substantial processing, observational data are used by research communities, their research groups and individual scientists, who interpret such primary data for their meaning in the context of research investigations. The result of interpretation is information—meaningful secondary or derived data—about the observed environment. Research infrastructures and research communities are thus essential to evolving uninterpreted observational data to information. In digital form, the classical bearer of information are the commonly known “(elaborated) data products,” for instance maps. In such form, meaning is generally implicit e.g., in map colour coding, and thus largely inaccessible to machines. The systematic acquisition, curation, possible publishing and further processing of information gained in observational data interpretation—as machine readable data and their machine readable meaning—is not common practice among environmental research infrastructures. For a use case in aerosol science, we elucidate these problems and present a Jupyter based prototype infrastructure that exploits a machine learning approach to interpretation and could support a research community in interpreting observational data and, more importantly, in curating and further using resulting information about a studied natural phenomenon.

2018

Assessment of air quality microsensors versus reference methods: The EuNetAir Joint Exercise – Part II

Borrego, Carlos; Ginja, Joao; Coutinho, Miguel; Ribeiro, Clara; Karatzas, Kostas; Sioumis, Th.; Katsifarakis, Nikos; Konstantinidis, Konstantinos; Vito, Saverio De; Esposito, Elena; Salvato, Maria; Smith, Paul D.; Andre, Nicolas; Gerard, Pierre; Francis, Laurent Alain; Castell, Nuria; Schneider, Philipp; Viana, Mar; Minguillón, María Cruz; Reimringer, Wolfhard; Otjes, Rene; Sicard, Oliver von; Pohle, Roland; Elen, Bart; Suriano, Domenico; Pfister, Valerio; Prato, Mario; Dipinto, S.; Penza, Michèle

2018

Atlantic multidecadal oscillation modulates the impacts of Arctic sea ice decline

Li, Fei; Orsolini, Yvan; Wang, Huijun; Gao, Yongqi; He, Shengping

The Arctic sea ice cover has been rapidly declining in the last two decades, concurrent with a shift in the Atlantic Multidecadal Oscillation (AMO) to its warm phase around 1996/1997. Here we use both observations and model simulations to investigate the modulation of the atmospheric impacts of the decreased sea ice cover in the Atlantic sector of the Arctic (AASIC) by the AMO. We find that the AASIC loss during a cold AMO phase induces increased Ural blocking activity, a southeastward‐extended snowpack, and a cold continent anomaly over Eurasia in December through northerly cold air advection and moisture transport from the Arctic. The increased Ural blocking activity and more extended Eurasian snowpack strengthen the upward propagation of planetary waves over the Siberian‐Pacific sector in the lower stratosphere and hence lead to a weakened stratospheric polar vortex and a negative Arctic Oscillation (AO) phase at the surface in February. However, corresponding to the AASIC loss during a warm AMO phase, one finds more widespread warming over the Arctic and a reduced snowpack over Northern Eurasia in December. The stratosphere‐troposphere coupling is suppressed in early winter and no negative AO anomaly is found in February. We suggest that the cold AMO phase is important to regulate the atmospheric response to AASIC decline, and our study provides insight to the ongoing debate on the connection between the Arctic sea ice and the AO.

2018

Assessing, quantifying and valuing the ecosystem services of coastal lagoons

Newton, Alice; Brito, Ana C.; Icely, John D.; Derolez, Valérie; Clara, Inês; Angus, Stewart; Schernewski, Gerard; Inácio, Miguel; Lillebø, Ana I.; Sousa, Ana Isabel; Béjaoui, Béchir; Solidoro, Cosimo; Tosic, Marko; Cañedo-Argüelles, Miguel; Yamamuro, Masumi; Reizopoulou, Sofia; Tseng, Hsiao-Chun; Donata, Canu; Roselli, Leonilde; Maanan, Mohamed; Cristina, Sónia; Ruiz-Fernández, Ana Carolina; Lima, Ricardo; Kjerfve, Björn; Rubio-Cisneros, Nadia; Perez-Ruzafa, Angel; Marcos, Concepción; Pastres, Roberto; Pranovi, Fabio; Snoussi, Maria; Turpie, Jane; Tuchkovenko, Yurii; Dyack, Brenda; Brookes, Justin; Povilanskas, Ramunas; Khokhlov, Valeriy

The natural conservation of coastal lagoons is important not only for their ecological importance, but also because of the valuable ecosystem services they provide for human welfare and wellbeing. Coastal lagoons are shallow semi-enclosed systems that support important habitats such as wetlands, mangroves, salt-marshes and seagrass meadows, as well as a rich biodiversity. Coastal lagoons are also complex social-ecological systems and the ecosystem services that lagoons deliver provide livelihoods, benefits wellbeing and welfare to humans. This study assessed, quantified and valued the ecosystem services of 32 coastal lagoons. The main findings of the study were: (i) the definitions of ecosystem services are still not generally accepted; (ii) the quantification of ecosystem services is made in many different ways, using different units; (iii) the evaluation in monetary terms of some ecosystem service is problematic, often relying on non-monetary evaluation methods; (iv) when ecosystem services are valued in monetary terms, this may represent very different human benefits; and, (v) different aspects of climate change, including increasing temperature (SST), sea-level rise (SLR) and changes in rainfall patterns threaten the valuable ecosystem services of coastal lagoons.

2018

CITI-SENSE Citizens' Observatories Architecture

Liu, Hai-Ying; Berre, Arne- Jørgen; Kobernus, Michael John; Fredriksen, Mirjam; Rombouts, Richard; Tamlin, Andrei; Cole-Hunter, Tom; Santiago, Leonardo; Bartonova, Alena

This paper introduces the architecture of the CITI-SENSE Citizens’ Observatories based on the ISO 19119 reference model. It describes the various parts of the architecture including boundary services with sensors and apps and data management services with the CITI-SENSE data model. It also describes the Web Feature Service (WFS) storage support and the reusable visualisation widgets used for both apps and web portals in various Citizens’ Observatories.

2018

An aerosol particle containing enriched uranium encountered in the remote upper troposphere

Murphy, D. M.; Froyd, K. D.; Apel, E.; Blake, D.; Evangeliou, Nikolaos; Hornbrook, R. S.; Peischl, J.; Ray, E.; Ryerson, T. B.; Thompson, C.; Stohl, Andreas

2018

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