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Found 9990 publications. Showing page 32 of 400:

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What do we know about the production and release of persistent organic pollutants in the global environment?

Li, Li; Cheng, Chengkang; Li, Dingsheng; Breivik, Knut; Abbasi, Golnoush; Li, Yi-Fan

Information on the global production and environmental releases of persistent organic pollutants (POPs) is of critical importance for regulating and eliminating these chemical substances of worldwide environmental and health concerns. Here, we conduct an extensive literature review to collect and curate quantitative information on the historical global production and multimedia environmental releases of 25 intentionally produced POPs. Our assembled data indicate that as of 2020, a cumulative total of 31 306 kilotonnes (kt) of the 25 POPs had been synthesized and commercialized worldwide, resulting in cumulative releases of 20 348 kt into the global environment. As of 2020, short-chain chlorinated paraffins were the most produced POP, with a historical global cumulative tonnage amounting to 8795 kt, whereas α-hexachlorocyclohexane (HCH) had the largest historical global cumulative environmental releases of 6567 kt among these 25 POPs. The 1970s witnessed the peak in the annual global production of the 25 investigated POPs. The United States and Europe used to be the hotspots of environmental releases of the 25 investigated POPs, notably in the 1960s and 1970s. By contrast, global environmental releases occurred primarily in China in the 2000s–2010s. Preliminary efforts are also made to integrate the production volume information with “hazard” attributes (persistence, bioaccumulation, toxicity, and long-range transport potential) in the evaluation of potential environmental impacts of the 25 POPs. The results show that dichlorodiphenyltrichloroethane (DDT) and polychlorinated biphenyls (PCBs) are potentially associated with higher environmental impacts than other POPs because they are among the top rankings in both the global cumulative production and hazard indicators. This work for the first time reveals the astonishing magnitudes of POP production and environmental releases in contemporary human history. It also underscores the importance of tonnage information in assessments of POPs, POP candidates, and other chemicals of emerging concern.

2023

Inverse Modeling of Subnational Scale CO2 Emissions Using Data from Denser Surface Observation Networks

Nayagam, Lorna Raja; Maksyutov, Shamil; Oda, Tomohiro; Achari, Rajesh Janardanan; Trisolini, Pamela; Zeng, Jiye; Kaiser, Johannes; Matsunaga, Tsuneo

2023

National N2O emissions (1980-2020) derived from multiple sources of data: magnitudes, trends and drivers

Pan, Naiqing; Tian, Hanqin; Pan, Shufen; Canadell, Josep G.; Thompson, Rona Louise; Ciais, Philippe; Davidson, Eric A.; Ito, Akihiko; Jackson, Robert B.; Jain, Atul K.; Joos, Fortunat; Kou-Giesbrecht, Sian; Lauerwald, Ronny; Li, Ya; Lu, Chaoqun; Millet, Dylan B.; Muntean, Marilena; Patra, Prabir K.; Qin, Xiaoyu; Regnier, Pierre; Shi, Hao; Sun, Qing; Tubiello, Francesco N.; Vuichard, Nicolas; Wells, Kelley C.; Wilson, Chris J.; Winiwarter, Wilfried; Yang, Jia; Yao, Yuanzhi; You, Yongfa; Zaehle, Sönke; Zhou, Feng; Zhu, Qing

2023

Circular economy for aquatic food systems: insights from a multiscale phosphorus flow analysis in Norway

Pandit, Avijit Vinayak; Dittrich, Nils Maximilian; Strand, Andrea Viken; Lozach, Loïs; Hernandez, Miguel Las Heras; Reitan, Kjell Inge; Mueller, Daniel Beat

As wild-caught fish become scarce, feed ingredients for farming fish, such as salmon, are increasingly sourced from agricultural plants that depend on mineral fertilizers. Since these fish are naturally carnivorous, they have difficulty digesting the phosphorus in plant-based feed. So additional phosphorus supplements are added to the feed, resulting in a disproportionate increase in mineral phosphorus use and emission. Aquatic food production is increasingly relying on agriculture and mineral phosphorus resources. The feed surplus and the excreta are seldom collected and recycled, leading to a massive loss of nutrients to water bodies and the seafloor, resulting in local risk for eutrophication. Norway currently produces more than half of the world’s Atlantic salmon, and it is set to increase production from currently 1.5 to 5 Mt. in 2050. This has large implications for feed supply and emissions globally. There is a lack of studies that analyze the phosphorus system in aquatic food production at a sufficient spatial and temporal granularity to effectively inform interventions for a more circular use of phosphorus. Here, we present a multi-scale phosphorus flow analysis at monthly resolution ranging between 2005 and 2021 for aquatic food production in Norway and quantitatively discuss the effectiveness of alternative strategies for improving resource efficiency. The results indicate that P emissions from aquaculture have nearly doubled in the period between 2005 and 2021. The P use efficiency (PUE) in Norwegian aquaculture was 19% in 2021. The addition of phytase to the feed could improve the PUE by 8% by reducing P supplements and emissions by 7 kt/y. The use of Integrated Multi-Trophic Aquaculture close to fish farming sites could absorb emissions by 4 kt/y by creating new marine food products. Sludge collection systems could reduce P emissions by 4 to 11 kt/y, depending on the technology. Using the sludge in local agriculture would exacerbate the current P accumulation in soils close to the coastline, given that the animal density in this region is already high. Hence, a large and sophisticated processing infrastructure will be needed to create transportable, high-quality secondary fertilizers for effective sludge recycling in regions with a P deficit.

2023

Estimating High Resolution Surface PM2.5 Over Europe Using Satellite AOD Datasets, CAMS Forecast and Machine Learning

Shetty, Shobitha; Schneider, Philipp; Stebel, Kerstin; Hamer, Paul David; Kylling, Arve; Berntsen, Terje Koren

2023

Underestimation of Anthropogenic Bromoform Emissions: Implications for Ozone Depletion

Jia, Yue; Davis, Sean M; Tegtmeier, Susann; Quack, Birgit; Pisso, Ignacio; Portmann, Robert W.; Rosenlof, Karen H.

2023

Distinctive Changes in Natural Aerosols Capable of Ice Nucleation Likely Linked to the Climate and Ecosystems in Svalbard

Tobo, Yutaka; Adachi, Kouji; Kawai, Kei; Matsui, Hitoshi; Ohata, Sho; Oshima, Naga; Kondo, Yutaka; Hermansen, Ove; Inoue, Jun; Koike, Makoto

2023

Arctic Tropospheric Ozone Trends

Law, Kathy S.; Hjorth, Jens Liengaard; Pernov, Jakob B.; Whaley, Cynthia; Skov, Henrik; Coen, Martine Collaud; Langner, Joakim; Arnold, Stephen R.; Tarasick, David; Christensen, Jesper; Deushi, Makoto; Effertz, Peter; Faluvegi, Greg; Gauss, Michael; Im, Ulas; Oshima, Naga; Petropavlovskikh, Irina; Plummer, David; Tsigaridis, Kostas; Tsyro, Svetlana; Solberg, Sverre; Turnock, Stephen

Observed trends in tropospheric ozone, an important air pollutant and short-lived climate forcer (SLCF), are estimated using available surface and ozonesonde profile data for 1993–2019, using a coherent methodology, and compared to modeled trends (1995–2015) from the Arctic Monitoring Assessment Program SLCF 2021 assessment. Increases in observed surface ozone at Arctic coastal sites, notably during winter, and concurrent decreasing trends in surface carbon monoxide, are generally captured by multi-model median trends. Wintertime increases are also estimated in the free troposphere at most Arctic sites, with decreases during spring months. Winter trends tend to be overestimated by the multi-model medians. Springtime surface ozone increases in northern coastal Alaska are not simulated while negative springtime trends in northern Scandinavia are not always reproduced. Possible reasons for observed changes and model performance are discussed including decreasing precursor emissions, changing ozone dry deposition, and variability in large-scale meteorology.

2023

A rise in HFC-23 emissions from eastern Asia since 2015

Park, Hyeri; Kim, Jooil; Choi, Haklim; Geum, Sohyeon; Kim, Yeaseul; Thompson, Rona Louise; Mühle, Jens; Salameh, Peter K.; Harth, Christina M.; Stanley, Kieran M.; O'Doherty, Simon; Fraser, Paul J.; Simmonds, Peter G.; Krummel, Paul B.; Weiss, Ray F.; Prinn, Ronald G.; Park, Sunyoung

Trifluoromethane (CHF3, HFC-23), one of the most potent greenhouse gases among hydrofluorocarbons (HFCs), is mainly emitted to the atmosphere as a by-product in the production of the ozone-depleting legacy refrigerant and chemical feedstock chlorodifluoromethane (CHClF2, HCFC-22). A recent study on atmospheric observation-based global HFC-23 emissions (top-down estimates) showed significant discrepancies over 2014–2017 between the increase in the observation-derived emissions and the 87 % emission reduction expected from capture and destruction processes of HFC-23 at HCFC-22 production facilities implemented by national phase-out plans (bottom-up emission estimates) (Stanley et al., 2020). However, the actual regions responsible for the increased emissions were not identified. Here, we estimate the regional top-down emissions of HFC-23 for eastern Asia based on in situ measurements at Gosan, South Korea, and show that the HFC-23 emissions from eastern China have increased from 5.0±0.4 Gg yr−1 in 2008 to 9.5±1.0 Gg yr−1 in 2019. The continuous rise since 2015 was contrary to the large emissions reduction reported under the Chinese hydrochlorofluorocarbons production phase-out management plan (HPPMP). The cumulative difference between top-down and bottom-up estimates for 2015–2019 in eastern China was  Gg, which accounts for 47±11 % of the global mismatch. Our analysis based on HCFC-22 production information suggests the HFC-23 emissions rise in eastern China is more likely associated with known HCFC-22 production facilities rather than the existence of unreported, unknown HCFC-22 production, and thus observed discrepancies between top-down and bottom-up emissions could be attributed to unsuccessful factory-level HFC-23 abatement and inaccurate quantification of emission reductions.

2023

The turbulent future brings a breath of fresh air

Stjern, Camilla Weum; Hodnebrog, Øivind; Myhre, Gunnar; Pisso, Ignacio

Ventilation of health hazardous aerosol pollution within the planetary boundary layer (PBL) – the lowest layer of the atmosphere – is dependent upon turbulent mixing, which again is closely linked to the height of the PBL. Here we show that emissions of both CO2 and absorbing aerosols such as black carbon influence the number of severe air pollution episodes through impacts on turbulence and PBL height. While absorbing aerosols cause increased boundary layer stability and reduced turbulence through atmospheric heating, CO2 has the opposite effect over land through surface warming. In future scenarios with increasing CO2 concentrations and reduced aerosol emissions, we find that around 10% of the world’s population currently living in regions with high pollution levels are likely to experience a particularly strong increase in turbulence and PBL height, and thus a reduction in intense pollution events. Our results highlight how these boundary layer processes provide an added positive impact of black carbon mitigation to human health.

2023

Evaluation of meso- and microplastic ingestion by the northern fulmar through a non-lethal sampling method

Collard, France; Strøm, Hallvard; Fayet, Marie-Océane; Gudmundsson, Fannar Theyr; Herzke, Dorte; Hotvedt, Ådne; Løchen, Arja; Malherbe, Cédric; Eppe, Gauthier; Gabrielsen, Geir W.

An increasing number of organisms from the polar regions are reported contaminated by plastic. Rarely a non-killing sampling method is used. In this study we wanted to assess plastic levels using stomach flushing and evaluate the method suitability for further research and monitoring. The stomach of 22 fulmars from Bjørnøya, Svalbard, were flushed with water in the field. On return to the laboratory, the regurgitated content was digested using potassium hydroxide. The extracted plastics were visually characterised and analysed with spectroscopy. Only three birds had plastics in their stomach, totaling 36 particles, most of them microplastics (< 5 mm). The plastic burdens are much lower than previously reported in Svalbard. The stomach flushing is assumed not to allow the collection of the gizzard content. This is a major limitation as most of the plastics accumulate in the fulmar's gizzard. However, the method is still useful for studies investigating plastic ingestion dynamics, allowing to sample the same individuals over time.

2023

Increased contribution of biomass burning to haze events in Shanghai since China’s clean air actions

Fang, Wenzheng; Evangeliou, Nikolaos; Eckhardt, Sabine; Xing, Ju; Zhang, Hailong; Xiao, Hang; Zhao, Meixun; Kim, Sang-Woo

High levels of East Asian black carbon (BC) aerosols affect ecological and environmental sustainability and contribute to climate warming. Nevertheless, the BC sources in China, after implementing clean air actions from 2013‒2017, are currently elusive due to a lack of observational constraints. Here we combine dual-isotope-constrained observations and chemical-transport modelling to quantify BC’s sources and geographical origins in Shanghai. Modelled BC concentrations capture the overall source trend from continental China and the outflow to the Pacific. Fossil sources dominate (~70%) BC in relatively clean summer. However, a striking increase in biomass burning (15‒30% higher in a fraction of biomass burning compared to summer and 2013/2014 winter), primarily attributable to residential emissions, largely contributes to wintertime BC (~45%) pollution. It highlights the increasing importance of residential biomass burning in the recent winter haze associated with >65% emissions from China’s central-east corridor. Our results suggest clearing the haze problem in China’s megacities and mitigating climate impact requires substantial reductions in regional residential emissions, besides reducing urban traffic and industry emissions.

2023

Nivåer av tungmetaller og PCBer i elgkjøtt fra Sør-Varanger 2020

Aspholm, Paul Eric; Beddari, Benedicte; Søvik, Ingrid; Fløistad, Ida Marie Bardalen; Englund, Monika Strasser; Enge, Ellen Katrin; Vadset, Marit; Heimstad, Eldbjørg Sofie; Hagen, Snorre

Under høstjakta på elg (Alces alces) i 2020 ble det tatt vevsprøver til analyser av tungmetaller og PCB. Tungmetallprøver ble tatt av 24 individer; 4 hunnkalver, 4 hannkalver, 3 hanner av åringer og 13 okser (voksne hanner). PCB analyser ble gjort av vevsprøver som ble tatt av 2 hunnkalver, 3 hannkalver, 2 hann-åringer og 9 okser (totalt 16 dyr). De felte dyrene har god geografisk spredning fra sør til nord og nord-øst i kommunen. Tungmetallene som ble analysert var krom (Cr), nikkel (Ni), kobber (Cu), sink (Zn), arsen (As), sølv (Ag), kadmium (Cd), tinn (Sn), bly (Pb) og kvikksølv (Hg). PCB ble analysert for 34 kongenere pluss sumPCB6 og sumPCB7. De fleste konsentrasjonene av tungmetallene var svært lave og flere var under deteksjonsgrensene. Ellers var det bare sporadiske lave forekomster av de 32 PCBene som ble funnet i noen av de undersøkte elgene. Det var bare heksaklorbensen som ble detektert i alle prøvene fra elgene).

NIBIO

2023

Air pollution situation in small towns, including winter resorts: a comparative study of three cases in Northern Europe

Tammekivi, Terje; Kaasik, Marko; Hamer, Paul David; Santos, Gabriela Sousa; Šteinberga, Iveta

In Europe, emissions of many air pollutants have decreased in recent decades, but there exist sites where concentrations of pollutants are still high and have become a public health problem. The air quality monitoring networks include urban stations in big cities and rural background stations. Main pollutants (SO2, NOx, CO, particulate matter) are measured automatically and reported on hourly basis, but there is very few research about air quality in small towns. The small towns are important transport nodes between cities and nowadays they are growing bigger, often being focused on seasonal tourism. In this paper, we try to understand the level of pollution in three small towns in Northern Europe, namely Otepää (Estonia), Lillehammer (Norway) and Saldus (Latvia) This research we point at seasonality of air pollution in towns related with winter sport activities, where the traffic flow increases in cold time simultaneously with heating season and higher prevalence of thermal inversions in atmospheric surface layer. Concentration peak of PM10 in Northern Europe appears in early spring, in snow thawing season and shortly after that. Even higher episodic concentrations may occur near unpaved streets in dry season. High seasonal variation of measured nitrogen dioxide concentrations was found in Lillehammer and Otepää, with remarkable contributions of traffic hotspots. This paper confirms that it is worth to study the air quality in small towns, furthermore, because air pollution levels and related public health concerns in small towns are not negligible.

2023

Approche générique pour l’acquisition de contraintes qualitatives

Belaid, Mohamed-Bachir; Belmecheri, Nassim; Gotlieb, Arnaud; Lazaar, Nadjib; Spieker, Helge

2023

Nasjonalt veikart for CO2M/CO2MVS

Kylling, Arve; Børke, Ragnhild; Lopez-Aparicio, Susana; Peters, Glen Philip; Stebel, Kerstin; Tarrasón, Leonor

På vegne av Norsk Romsenter har NILU – Norsk institutt for luftforskning og CICERO Senter for klimaforskning utarbeidet et veikart for hvordan Norge kan nyttiggjøre seg data fra CO2 Monitoring-satellittene (CO2M) og tjenesten CO2-emissions Monitoring and Verification Support Capacity (CO2MVS) i forvaltning, forskningsmiljøer og næringsliv. Veikartet avslutter med anbefalinger for veien videre for Norge vedrørende CO2M og CO2MVS.

NILU

2023

EMEP CCC update

Tørseth, Kjetil; Aas, Wenche

2023

The Composite Response of Traveling Planetary Waves in the Middle Atmosphere Surrounding Sudden Stratospheric Warmings through an Overreflection Perspective

Rhodes, Christian Todd; Limpasuvan, Varavut; Orsolini, Yvan Joseph Georges Emile G.

Traveling planetary waves surrounding sudden stratospheric warming events can result from direct propagation from below or in situ generation. They can have significant impacts on the circulation in the mesosphere and lower thermosphere. Our study runs a series of ensembles initialized from the Whole Atmosphere Community Climate Model, Version 4, nudged up to 50 km by six-hourly Modern-Era Retrospective Analysis for Research and Application, Version 2, reanalysis to compile a library of sudden stratospheric warming events. To our knowledge, we present the first composite or ensemble study that attempts to link direct propagation and in situ generation by evaluating the wave geometries associated with the overreflection perspective, a framework used to describe how planetary waves interact with critical and turning levels. The present study looks at the evolution of these interactions through the onset of sudden stratospheric warmings with an elevated stratopause or ES-SSWs. Robust and unique features of ES-SSWs are determined by employing an ensemble study that compares ES-SSWs with normal winters. Our study evaluates the production and impacts of westward-propagating, quasi-stationary, and eastward-propagating planetary waves surrounding ES-SSWs. Our results show that eastward-propagating planetary waves are generated within the westward stratospheric wind layer after ES-SSW onset which aids in restoring the eastward stratospheric wind. The interaction of quasi-stationary and westward-propagating waves with the westward stratospheric wind is explored from an overreflection perspective and reaffirms that westward-propagating planetary waves are produced from instabilities at the top of the westward stratospheric wind reversal.

2023

Low-Processing Data Enrichment and Calibration for PM2.5 Low-Cost Sensors

Stojanović, Danka B.; Kleut, Duška N.; Davidović, Miloš D.; Vito, Saverio De; Jovasević-Stojanović, Milena V.; Bartonova, Alena; Lepioufle, Jean-Marie

Particulate matter (PM) in air has been proven to be hazardous to human health. Here we focused on analysis of PM data we obtained from the same campaign which was presented in our previous study. Multivariate linear and random forest models were used for the calibration and analysis. In our linear regression model the inputs were PM, temperature and humidity measured with low-cost sensors, and the target was the reference PM measurements obtained from SEPA in the same timeframe.

2023

Safety-by-design and engineered nanomaterials: the need to move from theory to practice

Trump, Benjamin D.; Antunes, Dalila; Palma-Oliveira, José; Nelson, Andrew; Hudecova, Alexandra Misci; Rundén-Pran, Elise; Dusinska, Maria; Gispert, Ignasi; Resch, Susanne; Alfaro-Serrano, Beatriz; Afantitis, Antreas; Melagraki, Georgia; Tse, Edmund C. M.; Trump, Josh; Kohl, Yvonne; Linkov, Igor

As the governance of engineered nanomaterials (ENMs) evolves, innovations in the prevention, mitigation, management, and transfer of risk shape discussion of how nanotechnology may mature and reach various marketplaces. Safety-by-Design (SbD) is one leading concept that, while equally philosophy as well as risk-based practice, can uniquely help address lingering uncertainties and concerns stemming from regulatory evaluation of ENM risk across worker, consumer, and environmental safety. This paper provides a discussion on the SbD concept across different disciplines aiming to identify different approaches and needs to meet regulatory requirements—ultimately, we argue that SbD is evolving both to meet the needs and discourse of various disciplines, and to apply within differing marketplaces and national regulatory structures. Understanding how SbD has evolved within ENM can yield a more practical application and development of SbD, and help guide or unify national and international ENM governance around a core set of safety-driven principles.

2023

Physical and chemical processes driving remote seasonal atmospheric exposure to cyclic volatile methysiloxanes and short-chain chlorinated paraffins

Saify, Insam Al; Brandsma, Sicco H.; Mourik, Louise M. van; Eckhardt, Sabine; Bohlin-Nizzetto, Pernilla; Warner, Nicholas Alexander

2023

Troll observing network – for useful new data about Antarctica

Pedersen, Christina Alsvik; Njåstad, Birgit; Descamps, Sebastien; Hattermann, Tore; Hudson, Stephen; Flått, Stig; Aas, Wenche; Darelius, Elin Maria K.; Miloch, Wojciech Jacek; Schweitzer, Johannes; Storvold, Rune

2023

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